There are several in-Call activities available such as Adding a call note, assigning an activity and creating a follow-up task.

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Adding a Note Add a note while on a call.
Notes are saved to the call record and contact history.
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In Call Activity: Adding a Note


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Relate to Relate a note and activity to any Entity in Dynamics 365.
This could be any Case or Opportunity.
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In Call Activity: Relate to


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Create New record Create a new record while on a phone call e.g., Account, Contact, Lead, Case or Opportunity.
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In Call Activity: Create New Record


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Assign To Assign an activity or information to an existing record.
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In Call Activity: Assign To


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Follow-up Task Schedule a next call or other action and add it to your D365 calendar and reminders.
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In Call Activity: Follow-up Task